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Oxygen doping and interface engineering in O-MoS2&rGO heterostructure for efficient piezocatalytic dye degradation
Lu, Zhichao1; Bai, Yuanjuan1; Zhang, Shuaijie1; Li, Yaxuan1; Liu, Mingxuan; Fang, Ling2; Liu, Li3; Du, Kun; Liu, Gonggang1; Xu, Laiqiang
2024-06-17
摘要To further apply MoS2 as a promising non-noble catalyst for addressing environmental issues, its catalytic ability must be improved. As a result of the hetero-atom doping effect and varied structure phase of MoS2, we demonstrated excellent piezocatalysis for the degradation of methylene blue (MB) dye under stirring/ultrasonic catalyzed by MoS2. Compared with pristine MoS2 and O-doping MoS2 (O-MoS2), O-MoS2& reduced graphene oxide (O-MoS2&rGO) exhibits enhanced piezocatalytic activity. When the initial concentration of MB solution is <= 15 mg L-1, both stirring and ultrasonication can make the optimal O-MoS2&rGO composite to degrade the dye completely within 20 min. The experimental results have led to the proposal of a mechanism that elucidates the enhancement effect of rGO and O doping on the piezocatalytic performance of MoS2. This study highlights the significance of constructing heterostructure interfaces and the impact of hetero-atom doping on the promotion of piezocatalysis efficiency.
DOI10.1557/s43578-024-01361-1
发表期刊JOURNAL OF MATERIALS RESEARCH
ISSN0884-2914
页码10
通讯作者Bai, Yuanjuan(byj@alu.cqu.edu.cn) ; Fang, Ling(fangling@cigit.ac.cn) ; Hu, Jinbo(hjb1999@hotmail.com)
收录类别SCI
WOS记录号WOS:001249563300005
语种英语